The prolific actress, who initially shot to fame via Suicide Squad and The Wolf of Wall Street, has climbed aboard Quentin Tarantino's Once Upon a Time in Hollywood as Sharon Tate, one of five people killed by the Manson Family nearly 50 years ago. She wrote alongside the picture: "First look".
The A-list cast also includes Al Pacino as DiCaprio's character's agent, Burt Reynolds, Timothy Olyphant, Damian Lewis, Luke Perry, Emile Hirsch, Dakota Fanning, Clifton Collins, Keith Jefferson, and Nicholas Hammond.
In a statement the Kill Bill filmmaker said: "I couldn't be happier about the dynamic teaming of DiCaprio & Pitt as Rick & Cliff".
DiCaprio recently shared a sneak peek of his and Pitt's characters dressed in head-to-toe '60s styles.
The shot finds the duo standing side-by-side and leaning against a stone building, with DiCaprio in an orange jacket, yellow turtleneck and brown trousers, while Pitt sports a denim jacket, jeans and sunglasses.
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While the late actress' family members weren't always keen on the film, given the tragic circumstances, her sister Debra Tate recently gave Tarantino their blessing after the director approached her about the project.
"I've been working on this script for five years, as well as living in Los Angeles County most of my life, including in 1969, when I was 7 years old".
Sony have now moved Once Upon A Time In Hollywood's release date up by two weeks to 26 July.
The upcoming movie won't heavily focus on Sharon Tate's murder, that's just the backdrop of the story, but it was going to be released on the exact 50th anniversary of Tate's death - August 9, 2019.
Then along came Margot Robbie posting a snap at herself playing Sharon Tate in the upcoming drama (above). But considering that Rick's neighbor is Sharon Tate, the wife of famous (and infamous) film director Roman Polanski, their struggles may be short-lived - before they get a whole lot worse in a much bigger way.